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ity and excellent mechanical strength. Recently, a previous study has reported that single layer graphene grown via chemical vapour deposition (CVD) was patterned and transferred to a target surface by controlling the surface energy of the polydimethylsiloxane stamp. However, their applications are limited because of the challenge of CVD-graphene functionalization for devices such as chemical or bio-sensors. In addition, graphene-based layers patterned with a micron scale width on the surface of biocompatible silk fibroin thin films, which are not suitable for conventional CMOS processes such as the patterning or etching of substrates, have yet to be reported. Herein, we developed a soft lithographic patterning process via surface energy modification for advanced graphene-based flexible devices such as transistors or chemical sensors. Using this approach, the surface of a relief-patterned elastomeric stamp was functionalized with hydrophilic dimethyls
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